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- 1. Phys. Rev. B 71, 115205 (2005) , “Origin of the 6885-cm–1 luminescence lines in ZnO: Vanadium versus copper”, L. S. Vlasenko, G. D. Watkins, R. HelbigOptical detection of electron paramagnetic resonance reveals the I=7/2 EPR spectrum of V2+ in the sharp photoluminescence (PL) lines often observed at ~6885 cm1 in ZnO, which have universally been assumed previously to arise from copper. An alternative model for... (Read more)
- 2. Semiconductors 38, 31-35 (2004) , “Green Luminescence Band of Zinc Oxide Films Copper-Doped by Thermal Diffusion”, Ya. I. Alivov, M. V. Chukichev, V. A. NikitenkoHigh quality ZnO single-crystal films were doped with copper by thermal diffusion, and their luminescent properties were studied by cathodoluminescence spectroscopy. Doping with copper increases the intensity of the green-emission band of the cathodoluminescence spectrum, whose peak, width, and shape at 78 and 300 K remain unchanged. At 4.2 K, a pronounced phonon structure with a phonon energy of 72 meV is detected in the cathodoluminescence green-emission band of the doped samples. In this case, the phonon peaks feature a triplet fine structure instead of the doublet one generally observed. This feature is attributed to radiative recombination of acceptor excitons that are localized at copper atoms and interact with each one of the subbands of the ZnO valence band. An analysis of the experimental data on the film cathodoluminescence and comparative studies of luminescence and electron spin resonance in single crystals allow one to conclude that the uncontrollable copper impurity typically existing in ZnO is responsible for green-emission luminescence in this material. (Read more)
- 3. Appl. Phys. Lett. 81, 622 (2002) , “Role of copper in the green luminescence from ZnO crystals”, N. Y. Garces, L. Wang, L. Bai, N. C. Giles, L. E. Halliburton, G. CantwellElectron paramagnetic resonance (EPR), photoluminescence, and infrared optical absorption have been used to investigate a ZnO crystal before and after a thermal anneal for 1 h in air at 900 °C. The sample was an undoped high quality crystal grown by the chemical vapor transport method. In... (Read more)
- 4. Appl. Surf. Sci. 147, 85-93 (1999) , “Influence of trivalent metal ions on the surface structure of a copper-based catalyst for methanol synthesis”, Hong-Bo Chen, Dai-Wei Liao, La-Jia Yu, Yi-Ji Lin, Jun Yi, Hong-Bin Zhang and Khi-Rui TsaiThe method of doping trivalent metal ions into a copper-based catalyst for methanol synthesis is effective in modifying the surface structure of the catalyst. The promotion effect and its relation to catalytic activity for hydrogenation of CO to methanol after doping with trivalent metal ions such... (Read more)
- 5. Jpn. J. Appl. Phys. 38, L113 (1999) , “Yellow Emission from Zinc Oxide giving an Electron Spin Resonance Signal at g=1.96”, Naoki Ohashi, Tomokazu Nakata, Takashi Sekiguchi, Hideo Hosono, Masafumi Mizuguchi, Takaaki Tsurumi, Junzo Tanaka, Hajime HanedaZnO polycrystals doped with Li, Cu or Al were prepared by solid-state reactions and their cathodoluminescence (CL) and electron spin resonance (ESR) spectra were measured. A strong yellow emission centered at 2.0 eV was observed for the Al-doped specimen and its intensity was higher than that of... (Read more)
- 6. Solid State Commun. 26, 779-781 (1978) , “Motional effects in the EPR-spectrum of Cu-H-centers in ZnO”, D. ZwingelAt low temperatures, the EPR signal of a Cu2+ center is observed in ZnO single crystals doped both with copper and hydrogen. A clear effect of line narrowing on the copper hfs-lines is observed at T=16K. It is discussed in the model of a Cu-(OH) complex taking into account the thermally induced... (Read more)
- 7. Solid State Commun. 15, 1475-1479 (1974) , “Optical and paramagnetic properties of ZnO-Crystals simultaneously doped with copper and hydrogen”, E. Mollwo, G. Müller and D. ZwingelIn ZnO crystals, containing both Cu and H(D), we observe characteristic absorption peaks in the near i.r. and three new EPR signals. We explain these results by the formation of impurity complexes consisting of an OH center and one or two Cu ions. (Read more)
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